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Experimental study on the performance of hydrogen production from miniature methanol–steam reformer integrated with Swiss-roll type combustor for PEMFC

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  • Chein, Rei-Yu
  • Chen, Yen-Cho
  • Chang, Che-Ming
  • Chung, J.N.

Abstract

A miniature plate-type hydrogen production reactor using methanol as fuel was designed and tested. This reactor is composed of a catalytic combustor, vaporizer, reformer, and methanator. All components were fabricated on one piece of rectangular quartz glass plate 50mm×44mm×7mm in size. The combustor was fabricated on one side of the glass plate with a Swiss-roll type channel in which the Pt/Al2O3 particles were loaded in segmented form to catalyze the combustion. A spiral channel was fabricated on the other side of the plate and divided into three sections: a vaporizer for liquid methanol–water mixture vaporization, a reformer for methanol–steam reforming catalyzed by CuO/ZnO/Al2O3 particles and a methanator for carbon monoxide (CO) removal catalyzed by Ru/Al2O3 particles.

Suggested Citation

  • Chein, Rei-Yu & Chen, Yen-Cho & Chang, Che-Ming & Chung, J.N., 2013. "Experimental study on the performance of hydrogen production from miniature methanol–steam reformer integrated with Swiss-roll type combustor for PEMFC," Applied Energy, Elsevier, vol. 105(C), pages 86-98.
    • Handle: RePEc:eee:appene:v:105:y:2013:i:c:p:86-98
    DOI: 10.1016/j.apenergy.2012.12.040
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    References listed on IDEAS

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    1. Shirsat, V. & Gupta, A.K., 2011. "A review of progress in heat recirculating meso-scale combustors," Applied Energy, Elsevier, vol. 88(12), pages 4294-4309.
    2. Chein, Reiyu & Chen, Yen-Cho & Chung, J.N., 2013. "Numerical study of methanol–steam reforming and methanol–air catalytic combustion in annulus reactors for hydrogen production," Applied Energy, Elsevier, vol. 102(C), pages 1022-1034.
    3. Liu, Qibin & Hong, Hui & Yuan, Jianli & Jin, Hongguang & Cai, Ruixian, 2009. "Experimental investigation of hydrogen production integrated methanol steam reforming with middle-temperature solar thermal energy," Applied Energy, Elsevier, vol. 86(2), pages 155-162, February.
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    5. Perng, Shiang-Wuu & Wu, Horng-Wen, 2022. "Influence of inlet-nozzle and outlet-diffuser mounted in the plate-shape reactor on PEMFC net power output and methanol steam reforming performance," Applied Energy, Elsevier, vol. 323(C).
    6. Wang, Qing-Hui & Yang, Song & Zhou, Wei & Li, Jing-Rong & Xu, Zhi-Jia & Ke, Yu-Zhi & Yu, Wei & Hu, Guang-Hua, 2018. "Optimizing the porosity configuration of porous copper fiber sintered felt for methanol steam reforming micro-reactor based on flow distribution," Applied Energy, Elsevier, vol. 216(C), pages 243-261.
    7. Perng, Shiang-Wuu & Horng, Rong-Fang & Wu, Horng-Wen, 2017. "Effect of a diffuser on performance enhancement of a cylindrical methanol steam reformer by computational fluid dynamic analysis," Applied Energy, Elsevier, vol. 206(C), pages 312-328.
    8. Chen, Wei-Hsin & Guo, Yu-Zhi & Chen, Chih-Chun, 2018. "Methanol partial oxidation accompanied by heat recirculation in a Swiss-roll reactor," Applied Energy, Elsevier, vol. 232(C), pages 79-88.
    9. Ribeirinha, P. & Abdollahzadeh, M. & Sousa, J.M. & Boaventura, M. & Mendes, A., 2017. "Modelling of a high-temperature polymer electrolyte membrane fuel cell integrated with a methanol steam reformer cell," Applied Energy, Elsevier, vol. 202(C), pages 6-19.
    10. Wang, Yancheng & Liu, Haiyu & Mei, Deqing & Yu, Shizheng, 2022. "Direct ink writing of 3D SiC scaffold as catalyst support for thermally autonomous methanol steam reforming microreactor," Renewable Energy, Elsevier, vol. 187(C), pages 923-932.
    11. Chen, Wei-Hsin & Chen, Chia-Yang, 2020. "Water gas shift reaction for hydrogen production and carbon dioxide capture: A review," Applied Energy, Elsevier, vol. 258(C).
    12. Ribeirinha, P. & Abdollahzadeh, M. & Pereira, A. & Relvas, F. & Boaventura, M. & Mendes, A., 2018. "High temperature PEM fuel cell integrated with a cellular membrane methanol steam reformer: Experimental and modelling," Applied Energy, Elsevier, vol. 215(C), pages 659-669.
    13. Ribeirinha, P. & Abdollahzadeh, M. & Boaventura, M. & Mendes, A., 2017. "H2 production with low carbon content via MSR in packed bed membrane reactors for high-temperature polymeric electrolyte membrane fuel cell," Applied Energy, Elsevier, vol. 188(C), pages 409-419.
    14. Cheng, Chin-Hsiang & Huang, Yu-Xian & King, Shun-Chih & Lee, Chun-I & Leu, Chih-Hsing, 2014. "CFD (computational fluid dynamics)-based optimal design of a micro-reformer by integrating computational a fluid dynamics code using a simplified conjugate-gradient method," Energy, Elsevier, vol. 70(C), pages 355-365.
    15. Kim, Taegyu & Jo, Sungkwon & Song, Young-Hoon & Lee, Dae Hoon, 2014. "Synergetic mechanism of methanol–steam reforming reaction in a catalytic reactor with electric discharges," Applied Energy, Elsevier, vol. 113(C), pages 1692-1699.

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