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Shell-isolated nanoparticle-enhanced Raman spectroscopy

Author

Listed:
  • Jian Feng Li

    (State Key Laboratory of Physical Chemistry of Solid Surfaces and College of Chemistry and Chemical Engineering, Xiamen University)

  • Yi Fan Huang

    (State Key Laboratory of Physical Chemistry of Solid Surfaces and College of Chemistry and Chemical Engineering, Xiamen University)

  • Yong Ding

    (School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332–0245, USA)

  • Zhi Lin Yang

    (State Key Laboratory of Physical Chemistry of Solid Surfaces and College of Chemistry and Chemical Engineering, Xiamen University)

  • Song Bo Li

    (State Key Laboratory of Physical Chemistry of Solid Surfaces and College of Chemistry and Chemical Engineering, Xiamen University)

  • Xiao Shun Zhou

    (State Key Laboratory of Physical Chemistry of Solid Surfaces and College of Chemistry and Chemical Engineering, Xiamen University)

  • Feng Ru Fan

    (State Key Laboratory of Physical Chemistry of Solid Surfaces and College of Chemistry and Chemical Engineering, Xiamen University
    School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332–0245, USA)

  • Wei Zhang

    (State Key Laboratory of Physical Chemistry of Solid Surfaces and College of Chemistry and Chemical Engineering, Xiamen University)

  • Zhi You Zhou

    (State Key Laboratory of Physical Chemistry of Solid Surfaces and College of Chemistry and Chemical Engineering, Xiamen University)

  • De Yin Wu

    (State Key Laboratory of Physical Chemistry of Solid Surfaces and College of Chemistry and Chemical Engineering, Xiamen University)

  • Bin Ren

    (State Key Laboratory of Physical Chemistry of Solid Surfaces and College of Chemistry and Chemical Engineering, Xiamen University)

  • Zhong Lin Wang

    (School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, Georgia 30332–0245, USA)

  • Zhong Qun Tian

    (State Key Laboratory of Physical Chemistry of Solid Surfaces and College of Chemistry and Chemical Engineering, Xiamen University)

Abstract

Raman spectroscopy unleashed Surface-enhanced Raman scattering (SERS) spectroscopy is a powerful analytical technique able to detect substances down to single molecule level. Its applications are limited, however, because to realize a substantial Raman signal requires metal substrates that either have roughened surfaces or take the form of nanoparticles. An innovative approach is now demonstrated, where the substance under investigation, on a generic substrate, is covered by a layer of 'smart dust' consisting of gold nanoparticles coated by an ultrathin insulating shell of silica or alumina. The nanoparticles provide Raman signal amplification, and the coating keeps them separate from each other and from the probed substance. The new technique, termed SHINERS (shell-isolated nanoparticle-enhanced Raman spectroscopy), is demonstrated by probing pesticide residues on the surfaces of yeast cells and citrus fruits. It could be useful in materials science and the life sciences, as well as for the inspection of food safety, drugs, explosives and environmental pollutants.

Suggested Citation

  • Jian Feng Li & Yi Fan Huang & Yong Ding & Zhi Lin Yang & Song Bo Li & Xiao Shun Zhou & Feng Ru Fan & Wei Zhang & Zhi You Zhou & De Yin Wu & Bin Ren & Zhong Lin Wang & Zhong Qun Tian, 2010. "Shell-isolated nanoparticle-enhanced Raman spectroscopy," Nature, Nature, vol. 464(7287), pages 392-395, March.
    • Handle: RePEc:nat:nature:v:464:y:2010:i:7287:d:10.1038_nature08907
    DOI: 10.1038/nature08907
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    3. Fu Wan & Lingling Du & Weigen Chen & Pinyi Wang & Jianxin Wang & Haiyang Shi, 2017. "A Novel Method to Directly Analyze Dissolved Acetic Acid in Transformer Oil without Extraction Using Raman Spectroscopy," Energies, MDPI, vol. 10(7), pages 1-12, July.
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    11. Zhi Chang & Huijun Yang & Anqiang Pan & Ping He & Haoshen Zhou, 2022. "An improved 9 micron thick separator for a 350 Wh/kg lithium metal rechargeable pouch cell," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    12. Xiaoxia Chang & Sudarshan Vijay & Yaran Zhao & Nicholas J. Oliveira & Karen Chan & Bingjun Xu, 2022. "Understanding the complementarities of surface-enhanced infrared and Raman spectroscopies in CO adsorption and electrochemical reduction," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
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    14. Chao-Yu Li & Ming Chen & Shuai Liu & Xinyao Lu & Jinhui Meng & Jiawei Yan & Héctor D. Abruña & Guang Feng & Tianquan Lian, 2022. "Unconventional interfacial water structure of highly concentrated aqueous electrolytes at negative electrode polarizations," Nature Communications, Nature, vol. 13(1), pages 1-10, December.

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