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Antiferromagnetic order as the competing ground state in electron-doped Nd1.85Ce0.15CuO4

Author

Listed:
  • H. J. Kang

    (The University of Tennessee)

  • Pengcheng Dai

    (The University of Tennessee
    Oak Ridge National Laboratory)

  • J. W. Lynn

    (NIST Center for Neutron Research, National Institute of Standards and Technology)

  • M. Matsuura

    (Oak Ridge National Laboratory)

  • J. R. Thompson

    (The University of Tennessee
    Oak Ridge National Laboratory)

  • Shou-Cheng Zhang

    (Stanford University)

  • D. N. Argyriou

    (Hahn-Meitner-Institut)

  • Y. Onose

    (Spin Superstructure Project, ERATO, Japan Science and Technology)

  • Y. Tokura

    (Spin Superstructure Project, ERATO, Japan Science and Technology
    Correlated Electron Research Center
    University of Tokyo)

Abstract

Superconductivity in the high-transition-temperature (high-Tc) copper oxides competes with other possible ground states1,2. The physical explanation for superconductivity can be constrained by determining the nature of the closest competing ground state, and establishing if that state is universal among the high-Tc materials. Antiferromagnetism has been theoretically predicted3,4 to be the competing ground state. A competing ground state is revealed when superconductivity is destroyed by the application of a magnetic field, and antiferromagnetism has been observed in hole-doped materials under the influence of modest fields5,6,7,8,9,10,11,12. None of the previous experiments have revealed the quantum phase transition from the superconducting state to the antiferromagnetic state, because they failed to reach the upper critical field Bc2. Here we report the results of transport and neutron-scattering experiments on electron-doped Nd1.85Ce0.15CuO4 (refs 13, 14), where Bc2 can be reached15. The applied field reveals a static, commensurate, anomalously conducting long-range ordered antiferromagnetic state, in which the induced moment scales approximately linearly with the field strength until it saturates at Bc2. This and previous experiments on the hole-doped materials therefore establishes antiferromagnetic order as a competing ground state in the high-Tc copper oxide materials, irrespective of electron or hole doping.

Suggested Citation

  • H. J. Kang & Pengcheng Dai & J. W. Lynn & M. Matsuura & J. R. Thompson & Shou-Cheng Zhang & D. N. Argyriou & Y. Onose & Y. Tokura, 2003. "Antiferromagnetic order as the competing ground state in electron-doped Nd1.85Ce0.15CuO4," Nature, Nature, vol. 423(6939), pages 522-525, May.
  • Handle: RePEc:nat:nature:v:423:y:2003:i:6939:d:10.1038_nature01641
    DOI: 10.1038/nature01641
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