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Higgs transition from a magnetic Coulomb liquid to a ferromagnet in Yb2Ti2O7

Author

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  • Lieh-Jeng Chang

    (National Cheng Kung University
    Quantum Beam Science Directorate, Japan Atomic Energy Agency)

  • Shigeki Onoda

    (Condensed Matter Theory Laboratory, RIKEN)

  • Yixi Su

    (Jülich Centre for Neutron Science JCNS-FRM II, Forschungszentrum Jülich GmbH, Outstation at FRM II, Lichtenbergstrasse 1, D-85747 Garching, Germany.)

  • Ying-Jer Kao

    (National Taiwan University)

  • Ku-Ding Tsuei

    (National Synchrotron Radiation Research Center)

  • Yukio Yasui

    (Nagoya University, Furo-cho, Chikusa-ku, Nagoya 464-8602, Japan.
    Meiji University)

  • Kazuhisa Kakurai

    (Quantum Beam Science Directorate, Japan Atomic Energy Agency)

  • Martin Richard Lees

    (University of Warwick)

Abstract

In a class of frustrated magnets known as spin ice, magnetic monopoles emerge as classical defects and interact via the magnetic Coulomb law. With quantum-mechanical interactions, these magnetic charges are carried by fractionalized bosonic quasi-particles, spinons, which can undergo Bose–Einstein condensation through a first-order transition via the Higgs mechanism. Here, we report evidence of a Higgs transition from a magnetic Coulomb liquid to a ferromagnet in single-crystal Yb2Ti2O7. Polarized neutron scattering experiments show that the diffuse [111]-rod scattering and pinch-point features, which develop on cooling are suddenly suppressed below TC~0.21 K, where magnetic Bragg peaks and a full depolarization of the neutron spins are observed with thermal hysteresis, indicating a first-order ferromagnetic transition. Our results are explained on the basis of a quantum spin-ice model, whose high-temperature phase is effectively described as a magnetic Coulomb liquid, whereas the ground state shows a nearly collinear ferromagnetism with gapped spin excitations.

Suggested Citation

  • Lieh-Jeng Chang & Shigeki Onoda & Yixi Su & Ying-Jer Kao & Ku-Ding Tsuei & Yukio Yasui & Kazuhisa Kakurai & Martin Richard Lees, 2012. "Higgs transition from a magnetic Coulomb liquid to a ferromagnet in Yb2Ti2O7," Nature Communications, Nature, vol. 3(1), pages 1-7, January.
  • Handle: RePEc:nat:natcom:v:3:y:2012:i:1:d:10.1038_ncomms1989
    DOI: 10.1038/ncomms1989
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