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Coherence in resonance fluorescence

Author

Listed:
  • Xu-Jie Wang

    (Beijing Academy of Quantum Information Sciences)

  • Guoqi Huang

    (Beijing Academy of Quantum Information Sciences
    Beijing University of Posts and Telecommunications)

  • Ming-Yang Li

    (Nanjing University)

  • Yuan-Zhuo Wang

    (Nanjing University)

  • Li Liu

    (Beijing Academy of Quantum Information Sciences)

  • Bang Wu

    (Beijing Academy of Quantum Information Sciences)

  • Hanqing Liu

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Haiqiao Ni

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Zhichuan Niu

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Weijie Ji

    (Beijing Academy of Quantum Information Sciences)

  • Rongzhen Jiao

    (Beijing University of Posts and Telecommunications)

  • Hua-Lei Yin

    (Beijing Academy of Quantum Information Sciences
    Nanjing University
    Renmin University of China)

  • Zhiliang Yuan

    (Beijing Academy of Quantum Information Sciences)

Abstract

Resonance fluorescence of a two-level emitter displays persistently anti-bunching irrespective of the excitation intensity, but inherits the driving laser’s linewidth under weak monochromatic excitation. These properties are commonly explained in terms of two disjoined pictures, i.e., the emitter’s single photon saturation or passively scattering light. Here, we propose a unified model that treats all fluorescence photons as spontaneous emission, one at a time, and can explain simultaneously both the spectral and correlation properties of the emission. We theoretically derive the excitation power dependencies, measurable at the single-photon incidence level, of the first-order coherence of the whole resonance fluorescence and super-bunching of the spectrally filtered, followed by experimental confirmation on a semiconductor quantum dot micro-pillar device. Furthermore, our model explains peculiar coincidence bunching observed in phase-dependent two-photon interference experiments. Our work provides an intuitive understanding of coherent light-matter interaction and may stimulate new applications.

Suggested Citation

  • Xu-Jie Wang & Guoqi Huang & Ming-Yang Li & Yuan-Zhuo Wang & Li Liu & Bang Wu & Hanqing Liu & Haiqiao Ni & Zhichuan Niu & Weijie Ji & Rongzhen Jiao & Hua-Lei Yin & Zhiliang Yuan, 2025. "Coherence in resonance fluorescence," Nature Communications, Nature, vol. 16(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:16:y:2025:i:1:d:10.1038_s41467-025-61884-x
    DOI: 10.1038/s41467-025-61884-x
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    References listed on IDEAS

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    1. Clemens Matthiesen & Martin Geller & Carsten H. H. Schulte & Claire Le Gall & Jack Hansom & Zhengyong Li & Maxime Hugues & Edmund Clarke & Mete Atatüre, 2013. "Phase-locked indistinguishable photons with synthesized waveforms from a solid-state source," Nature Communications, Nature, vol. 4(1), pages 1-6, June.
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