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Spectrally sharp magnetic excitations above the critical temperature in a frustrated Weyl semimetal

Author

Listed:
  • Michael Terilli

    (Rutgers University)

  • Xun Jia

    (Argonne National Laboratory
    Chinese Academy of Sciences)

  • Xiaoran Liu

    (Rutgers University
    Chinese Academy of Sciences)

  • Pontus Laurell

    (University of Tennessee)

  • Ana-Marija Nedić

    (University of Minnesota
    University of Minnesota)

  • Yueqing Chang

    (Rutgers University
    Rutgers University)

  • Tsung-Chi Wu

    (Rutgers University)

  • Huyongqing Chen

    (Boston University)

  • Hongze Li

    (University of Texas at Austin)

  • Mary H. Upton

    (Argonne National Laboratory)

  • Jungho Kim

    (Argonne National Laboratory)

  • Jong-Woo Kim

    (Argonne National Laboratory)

  • Philip J. Ryan

    (Argonne National Laboratory)

  • Christie Nelson

    (Brookhaven National Laboratory)

  • Jianshi Zhou

    (University of Texas at Austin)

  • Mikhail Kareev

    (Rutgers University)

  • Wanzheng Hu

    (Boston University
    Boston University
    Boston University)

  • Jedediah H. Pixley

    (Rutgers University
    Rutgers University
    Flatiron Institute)

  • Gregory A. Fiete

    (Northeastern University
    Massachusetts Institute of Technology)

  • Yue Cao

    (Argonne National Laboratory
    University of Chicago)

  • Jak Chakhalian

    (Rutgers University)

Abstract

The rare-earth α-pyrochlore iridates are a prospective class of conducting frustrated magnets where electronic correlations, large spin-orbit coupling, and geometrical frustration interplay, leading to a rich set of magnetic and electronic phases. Despite their intriguing properties, the magnetic order and excitations in this fundamental class of topological quantum materials remain poorly understood due to challenges in growing large single crystals and insufficient microscopic information on their temperature-dependent phases. Here, by combining state-of-the-art thin-film synthesis, resonant elastic and inelastic X-ray scattering, spin wave analysis, and dynamical spin susceptibility calculations, we unequivocally reveal the presence of spectrally sharp, gapped magnetic excitations in Y2Ir2O7 that surprisingly persist well above the Néel transition temperature, signaling the presence of a quasi-universal regime connected to fluctuations on frustrated lattices. This finding implies the existence of a highly unusual cooperative paramagnetic (CP) phase above the ordering temperature and offers an explanation for the puzzling high-temperature magnetic behavior observed across the family of metallic pyrochlore crystals. Understanding such magnetic excitations at technologically relevant temperatures opens up possibilities for novel topological spintronic devices.

Suggested Citation

  • Michael Terilli & Xun Jia & Xiaoran Liu & Pontus Laurell & Ana-Marija Nedić & Yueqing Chang & Tsung-Chi Wu & Huyongqing Chen & Hongze Li & Mary H. Upton & Jungho Kim & Jong-Woo Kim & Philip J. Ryan & , 2025. "Spectrally sharp magnetic excitations above the critical temperature in a frustrated Weyl semimetal," Nature Communications, Nature, vol. 16(1), pages 1-11, December.
  • Handle: RePEc:nat:natcom:v:16:y:2025:i:1:d:10.1038_s41467-025-61752-8
    DOI: 10.1038/s41467-025-61752-8
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