IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v16y2025i1d10.1038_s41467-025-61752-8.html
   My bibliography  Save this article

Spectrally sharp magnetic excitations above the critical temperature in a frustrated Weyl semimetal

Author

Listed:
  • Michael Terilli

    (Rutgers University)

  • Xun Jia

    (Argonne National Laboratory
    Chinese Academy of Sciences)

  • Xiaoran Liu

    (Rutgers University
    Chinese Academy of Sciences)

  • Pontus Laurell

    (University of Tennessee)

  • Ana-Marija Nedić

    (University of Minnesota
    University of Minnesota)

  • Yueqing Chang

    (Rutgers University
    Rutgers University)

  • Tsung-Chi Wu

    (Rutgers University)

  • Huyongqing Chen

    (Boston University)

  • Hongze Li

    (University of Texas at Austin)

  • Mary H. Upton

    (Argonne National Laboratory)

  • Jungho Kim

    (Argonne National Laboratory)

  • Jong-Woo Kim

    (Argonne National Laboratory)

  • Philip J. Ryan

    (Argonne National Laboratory)

  • Christie Nelson

    (Brookhaven National Laboratory)

  • Jianshi Zhou

    (University of Texas at Austin)

  • Mikhail Kareev

    (Rutgers University)

  • Wanzheng Hu

    (Boston University
    Boston University
    Boston University)

  • Jedediah H. Pixley

    (Rutgers University
    Rutgers University
    Flatiron Institute)

  • Gregory A. Fiete

    (Northeastern University
    Massachusetts Institute of Technology)

  • Yue Cao

    (Argonne National Laboratory
    University of Chicago)

  • Jak Chakhalian

    (Rutgers University)

Abstract

The rare-earth α-pyrochlore iridates are a prospective class of conducting frustrated magnets where electronic correlations, large spin-orbit coupling, and geometrical frustration interplay, leading to a rich set of magnetic and electronic phases. Despite their intriguing properties, the magnetic order and excitations in this fundamental class of topological quantum materials remain poorly understood due to challenges in growing large single crystals and insufficient microscopic information on their temperature-dependent phases. Here, by combining state-of-the-art thin-film synthesis, resonant elastic and inelastic X-ray scattering, spin wave analysis, and dynamical spin susceptibility calculations, we unequivocally reveal the presence of spectrally sharp, gapped magnetic excitations in Y2Ir2O7 that surprisingly persist well above the Néel transition temperature, signaling the presence of a quasi-universal regime connected to fluctuations on frustrated lattices. This finding implies the existence of a highly unusual cooperative paramagnetic (CP) phase above the ordering temperature and offers an explanation for the puzzling high-temperature magnetic behavior observed across the family of metallic pyrochlore crystals. Understanding such magnetic excitations at technologically relevant temperatures opens up possibilities for novel topological spintronic devices.

Suggested Citation

  • Michael Terilli & Xun Jia & Xiaoran Liu & Pontus Laurell & Ana-Marija Nedić & Yueqing Chang & Tsung-Chi Wu & Huyongqing Chen & Hongze Li & Mary H. Upton & Jungho Kim & Jong-Woo Kim & Philip J. Ryan & , 2025. "Spectrally sharp magnetic excitations above the critical temperature in a frustrated Weyl semimetal," Nature Communications, Nature, vol. 16(1), pages 1-11, December.
  • Handle: RePEc:nat:natcom:v:16:y:2025:i:1:d:10.1038_s41467-025-61752-8
    DOI: 10.1038/s41467-025-61752-8
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-025-61752-8
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-025-61752-8?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Lichen Wang & Guanhong He & Zichen Yang & Mirian Garcia-Fernandez & Abhishek Nag & Kejin Zhou & Matteo Minola & Matthieu Le Tacon & Bernhard Keimer & Yingying Peng & Yuan Li, 2022. "Paramagnons and high-temperature superconductivity in a model family of cuprates," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    2. Mariam Kavai & Joel Friedman & Kyle Sherman & Mingda Gong & Ioannis Giannakis & Samad Hajinazar & Haoyu Hu & Sarah E. Grefe & Justin Leshen & Qiu Yang & Satoru Nakatsuji & Aleksey N. Kolmogorov & Qimi, 2021. "Inhomogeneous Kondo-lattice in geometrically frustrated Pr2Ir2O7," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    3. C. Castelnovo & R. Moessner & S. L. Sondhi, 2008. "Magnetic monopoles in spin ice," Nature, Nature, vol. 451(7174), pages 42-45, January.
    4. Kentaro Ueda & Taekoo Oh & Bohm-Jung Yang & Ryoma Kaneko & Jun Fujioka & Naoto Nagaosa & Yoshinori Tokura, 2017. "Magnetic-field induced multiple topological phases in pyrochlore iridates with Mott criticality," Nature Communications, Nature, vol. 8(1), pages 1-7, August.
    5. Yao Shen & Yao-Dong Li & H. C. Walker & P. Steffens & M. Boehm & Xiaowen Zhang & Shoudong Shen & Hongliang Wo & Gang Chen & Jun Zhao, 2018. "Fractionalized excitations in the partially magnetized spin liquid candidate YbMgGaO4," Nature Communications, Nature, vol. 9(1), pages 1-7, December.
    6. W. He & Y. Shen & K. Wohlfeld & J. Sears & J. Li & J. Pelliciari & M. Walicki & S. Johnston & E. Baldini & V. Bisogni & M. Mitrano & M. P. M. Dean, 2024. "Magnetically propagating Hund’s exciton in van der Waals antiferromagnet NiPS3," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    7. Takeshi Kondo & M. Nakayama & R. Chen & J. J. Ishikawa & E.-G. Moon & T. Yamamoto & Y. Ota & W. Malaeb & H. Kanai & Y. Nakashima & Y. Ishida & R. Yoshida & H. Yamamoto & M. Matsunami & S. Kimura & N. , 2015. "Quadratic Fermi node in a 3D strongly correlated semimetal," Nature Communications, Nature, vol. 6(1), pages 1-8, December.
    8. Dirk Wulferding & Youngsu Choi & Seung-Hwan Do & Chan Hyeon Lee & Peter Lemmens & Clément Faugeras & Yann Gallais & Kwang-Yong Choi, 2020. "Magnon bound states versus anyonic Majorana excitations in the Kitaev honeycomb magnet α-RuCl3," Nature Communications, Nature, vol. 11(1), pages 1-7, December.
    9. B. A. Trump & S. M. Koohpayeh & K. J. T. Livi & J.-J. Wen & K. E. Arpino & Q. M. Ramasse & R. Brydson & M. Feygenson & H. Takeda & M. Takigawa & K. Kimura & S. Nakatsuji & C. L. Broholm & T. M. McQuee, 2018. "Universal geometric frustration in pyrochlores," Nature Communications, Nature, vol. 9(1), pages 1-10, December.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. J. Guo & P. Ghosh & D. Hill & Y. Chen & L. Stingaciu & P. Zolnierczuk & C. A. Ullrich & D. K. Singh, 2023. "Persistent dynamic magnetic state in artificial honeycomb spin ice," Nature Communications, Nature, vol. 14(1), pages 1-6, December.
    2. Robert Puttock & Ingrid M. Andersen & Christophe Gatel & Bumsu Park & Mark C. Rosamond & Etienne Snoeck & Olga Kazakova, 2022. "Defect-induced monopole injection and manipulation in artificial spin ice," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    3. Xiaoran Liu & Jong-Woo Kim & Yao Wang & Michael Terilli & Xun Jia & Mikhail Kareev & Shiyu Peng & Fangdi Wen & Tsung-Chi Wu & Huyongqing Chen & Wanzheng Hu & Mary H. Upton & Jungho Kim & Yongseong Cho, 2024. "Chiral spin-liquid-like state in pyrochlore iridate thin films," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    4. Xiaoyu Zhang & Ayhan Duzgun & Yuyang Lao & Shayaan Subzwari & Nicholas S. Bingham & Joseph Sklenar & Hilal Saglam & Justin Ramberger & Joseph T. Batley & Justin D. Watts & Daniel Bromley & Rajesh V. C, 2021. "String Phase in an Artificial Spin Ice," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
    5. D. Subires & A. Kar & A. Korshunov & C. A. Fuller & Yi Jiang & H. Hu & D. Călugăru & C. McMonagle & C. Yi & S. Roychowdhury & W. Schnelle & C. Shekhar & J. Strempfer & A. Jana & I. Vobornik & J. Dai &, 2025. "Frustrated charge density wave and quasi-long-range bond-orientational order in the magnetic kagome FeGe," Nature Communications, Nature, vol. 16(1), pages 1-11, December.
    6. Michael Saccone & Francesco Caravelli & Kevin Hofhuis & Scott Dhuey & Andreas Scholl & Cristiano Nisoli & Alan Farhan, 2023. "Real-space observation of ergodicity transitions in artificial spin ice," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    7. Daniel Lozano-Gómez & Yasir Iqbal & Matthias Vojta, 2024. "A classical chiral spin liquid from chiral interactions on the pyrochlore lattice," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    8. Lun-Hui Hu & Rui-Xing Zhang, 2023. "Topological superconducting vortex from trivial electronic bands," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    9. Zhi-Hao Cui & Junjie Yang & Johannes Tölle & Hong-Zhou Ye & Shunyue Yuan & Huanchen Zhai & Gunhee Park & Raehyun Kim & Xing Zhang & Lin Lin & Timothy C. Berkelbach & Garnet Kin-Lic Chan, 2025. "Ab initio quantum many-body description of superconducting trends in the cuprates," Nature Communications, Nature, vol. 16(1), pages 1-10, December.
    10. Youngsu Choi & Suheon Lee & Je-Ho Lee & Seungyeol Lee & Maeng-Je Seong & Kwang-Yong Choi, 2021. "Bosonic spinons in anisotropic triangular antiferromagnets," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    11. Alejandro Lopez-Bezanilla & Jack Raymond & Kelly Boothby & Juan Carrasquilla & Cristiano Nisoli & Andrew D. King, 2023. "Kagome qubit ice," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    12. Arthur Penty & Johannes H. Jensen & Ida Breivik & Anders Strømberg & Erik Folven & Gunnar Tufte, 2025. "Controllable gliders in a nanomagnetic metamaterial," Nature Communications, Nature, vol. 16(1), pages 1-11, December.
    13. Xu-Guang Zhou & Han Li & Yasuhiro H. Matsuda & Akira Matsuo & Wei Li & Nobuyuki Kurita & Gang Su & Koichi Kindo & Hidekazu Tanaka, 2023. "Possible intermediate quantum spin liquid phase in α-RuCl3 under high magnetic fields up to 100 T," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    14. Han Zhang & Chengkun Xing & Kyle Noordhoek & Zhaoyu Liu & Tianhao Zhao & Lukas Horák & Qing Huang & Lin Hao & Junyi Yang & Shashi Pandey & Elbio Dagotto & Zhigang Jiang & Jiun-Haw Chu & Yan Xin & Eun , 2023. "Anomalous magnetoresistance by breaking ice rule in Bi2Ir2O7/Dy2Ti2O7 heterostructure," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    15. Qiang Gao & Shiyu Fan & Qisi Wang & Jiarui Li & Xiaolin Ren & Izabela Biało & Annabella Drewanowski & Pascal Rothenbühler & Jaewon Choi & Ronny Sutarto & Yao Wang & Tao Xiang & Jiangping Hu & Ke-Jin Z, 2024. "Magnetic excitations in strained infinite-layer nickelate PrNiO2 films," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    16. M. J. Pearce & K. Götze & A. Szabó & T. S. Sikkenk & M. R. Lees & A. T. Boothroyd & D. Prabhakaran & C. Castelnovo & P. A. Goddard, 2022. "Magnetic monopole density and antiferromagnetic domain control in spin-ice iridates," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    17. Cisternas, Jaime & Concha, Andrés, 2024. "Searching nontrivial magnetic equilibria using the deflated Newton method," Chaos, Solitons & Fractals, Elsevier, vol. 179(C).
    18. Taiki Uehara & Takumi Ohtsuki & Masafumi Udagawa & Satoru Nakatsuji & Yo Machida, 2022. "Phonon thermal Hall effect in a metallic spin ice," Nature Communications, Nature, vol. 13(1), pages 1-8, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:16:y:2025:i:1:d:10.1038_s41467-025-61752-8. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.