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Realization of Kagome Kondo lattice

Author

Listed:
  • Boqin Song

    (Chinese Academy of Sciences)

  • Yuyang Xie

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Wei-Jian Li

    (Nanjing University)

  • Hui Liu

    (Chinese Academy of Sciences)

  • Jing Chen

    (Chinese Academy of Sciences)

  • Shangjie Tian

    (Renmin University of China)

  • Xing Zhang

    (Chinese Academy of Sciences)

  • Qinghong Wang

    (Chinese Academy of Sciences)

  • Xintong Li

    (Chinese Academy of Sciences)

  • Hechang Lei

    (Renmin University of China)

  • Qinghua Zhang

    (Chinese Academy of Sciences)

  • Jian-gang Guo

    (Chinese Academy of Sciences)

  • Lin Zhao

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Shun-Li Yu

    (Nanjing University)

  • Xingjiang Zhou

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Xiaolong Chen

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Tianping Ying

    (Chinese Academy of Sciences)

Abstract

The Kondo lattice, describing a grid of the local magnetic moments coupling to itinerant electrons, is a fertile ground of strongly correlated states in condensed matter physics. While the Kagome lattice has long been predicted to host Kondo physics with exotic magnetism and nontrivial topology, no experimental realization has been achieved to the best of our knowledge. Here, we report the discovery of CsCr6Sb6, a van der Waals-like Kagome Kondo lattice featuring extremely flat, isolated bands at the Fermi level that composed entirely of Cr-3d electrons. We observe heavy fermions with the effective mass over 100 times greater than those of its vanadium counterpart. We also observe Kondo insulating behavior in an ultra-low carrier density of 1019 cm-3 and dimensionality-induced Kondo breakdown. Counterintuitively, mechanical exfoliation of the frustrated bulk reveals hidden A-type antiferromagnetism with even-odd layer-dependent anomalous Hall effect. The realization of Kondo physics in Kagome lattice opens avenues for exploring diverse quantum criticalities in a strongly-correlated frustrated system.

Suggested Citation

  • Boqin Song & Yuyang Xie & Wei-Jian Li & Hui Liu & Jing Chen & Shangjie Tian & Xing Zhang & Qinghong Wang & Xintong Li & Hechang Lei & Qinghua Zhang & Jian-gang Guo & Lin Zhao & Shun-Li Yu & Xingjiang , 2025. "Realization of Kagome Kondo lattice," Nature Communications, Nature, vol. 16(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:16:y:2025:i:1:d:10.1038_s41467-025-60785-3
    DOI: 10.1038/s41467-025-60785-3
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