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Experimental Study on Direct and Indirect Carbonation of Fly Ash from Fluidized Bed Combustion of Lignite

Author

Listed:
  • Marek Tańczyk

    (Institute of Chemical Engineering, Polish Academy of Sciences, ul. Bałtycka 5, 44-100 Gliwice, Poland)

  • Jolanta Jaschik

    (Institute of Chemical Engineering, Polish Academy of Sciences, ul. Bałtycka 5, 44-100 Gliwice, Poland)

  • Andrzej Kołodziej

    (Institute of Chemical Engineering, Polish Academy of Sciences, ul. Bałtycka 5, 44-100 Gliwice, Poland
    Faculty of Civil Engineering and Architecture, Opole University of Technology, ul. Katowicka 48, 45-061 Opole, Poland)

  • Anna Pawlaczyk-Kurek

    (Institute of Chemical Engineering, Polish Academy of Sciences, ul. Bałtycka 5, 44-100 Gliwice, Poland)

  • Aleksandra Janusz-Cygan

    (Institute of Chemical Engineering, Polish Academy of Sciences, ul. Bałtycka 5, 44-100 Gliwice, Poland)

  • Łukasz Hamryszak

    (Institute of Chemical Engineering, Polish Academy of Sciences, ul. Bałtycka 5, 44-100 Gliwice, Poland)

Abstract

The research problem was to determine the possibility of aqueous mineral carbonation using fly ash from lignite fluidized bed combustion. Both direct and indirect routes were used. The innovative nature of the research consisted of conducting experiments at atmospheric pressure and ambient temperature (20 °C). The synthetic gas mixture with composition analogical to the flue gas (nitrogen and up to 16 vol.% of carbon dioxide) was used. The experiments proved that almost all CO 2 from the gas was chemically bound at pH > 12. The sequestration capacity of studied fly ash is about 55–76 g CO 2 per 1 kg of ash in the case of the indirect method, and 80–95 g CO 2 per 1 kg of ash for the direct route. These values are similar to those presented in the literature, but unlike most publications, they were obtained under ambient conditions, which can significantly reduce the costs of the process.

Suggested Citation

  • Marek Tańczyk & Jolanta Jaschik & Andrzej Kołodziej & Anna Pawlaczyk-Kurek & Aleksandra Janusz-Cygan & Łukasz Hamryszak, 2025. "Experimental Study on Direct and Indirect Carbonation of Fly Ash from Fluidized Bed Combustion of Lignite," Energies, MDPI, vol. 18(19), pages 1-21, September.
    • Handle: RePEc:gam:jeners:v:18:y:2025:i:19:p:5059-:d:1756424
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    References listed on IDEAS

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    1. Mehdi Azadi & Mansour Edraki & Faezeh Farhang & Jiwhan Ahn, 2019. "Opportunities for Mineral Carbonation in Australia’s Mining Industry," Sustainability, MDPI, vol. 11(5), pages 1-21, February.
    2. Lackner, Klaus S. & Wendt, Christopher H. & Butt, Darryl P. & Joyce, Edward L. & Sharp, David H., 1995. "Carbon dioxide disposal in carbonate minerals," Energy, Elsevier, vol. 20(11), pages 1153-1170.
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