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Non-linear response of electrode–electrolyte interface at high current density

Author

Listed:
  • Ruiz, G.A.
  • Felice, C.J.
  • Valentinuzzi, M.E.

Abstract

A distributed parameter non-linear circuit is presented as fractal model of an electrode–electrolyte interface. It includes the charge transfer resistance and the double layer capacitance at each fractal level. The circuit explains the linear behavior of its series equivalent resistance Req with signals of amplitudes <20mV and constant frequency; however, for amplitudes beyond that limit, non-linearitiy is manifested in the dc component of the Req Fourier spectrum. As a consequence, both the equivalent resistance and reactance drop with voltage, facts reported experimentally by other authors.

Suggested Citation

  • Ruiz, G.A. & Felice, C.J. & Valentinuzzi, M.E., 2005. "Non-linear response of electrode–electrolyte interface at high current density," Chaos, Solitons & Fractals, Elsevier, vol. 25(3), pages 649-654.
    • Handle: RePEc:eee:chsofr:v:25:y:2005:i:3:p:649-654
    DOI: 10.1016/j.chaos.2004.11.029
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    Cited by:

    1. Ruiz, G. & Felice, C.J., 2007. "Non-linear response of an electrode–electrolyte interface impedance with the frequency," Chaos, Solitons & Fractals, Elsevier, vol. 31(2), pages 327-335.
    2. Felice, Carmelo José & Ruiz, Gabriel Alfredo, 2016. "Differential equation of a fractal electrode–electrolyte interface," Chaos, Solitons & Fractals, Elsevier, vol. 84(C), pages 81-87.

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