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Analytical approximation of a self-oscillatory reaction system using the Laplace-Borel transform

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  • Zhai, Chi
  • Sun, Wei

Abstract

Time-symmetry breaking bifurcations cause an open system to generate complex structures/patterns, prompting the study of far-from-equilibrium and nonlinear thermodynamics. Specifically, thegeneration of self-organized chemical-wave patterns by the Belousov-Zhabotinsky reaction attractedattention from the academic community, assimilar structureswidely exist in the chemical/biological environment. However, theoretical fundamentals of these self-oscillatory structures are yet to be adequately addressed. This paper introducesa frequency-domain method for approximating the Belousov-Zhabotinskyreaction system.The nonlinear dynamics of the oscillator is estimated using the Laplace-Borel transform, which is an extension of the Laplace transform andutilizesfunctional expansions to approximate the nonlinear terms in the dynamic system.The method is applied to theBelousov-Zhabotinskyreaction model to yieldamplitude, frequency and stability characteristics near theAndronov-Hopf bifurcation points. By studying the emergence of self-oscillatory patternsusing this analytical method, new insights towardsfar-from-equilibrium and nonlinearthermodynamics are explored.

Suggested Citation

  • Zhai, Chi & Sun, Wei, 2021. "Analytical approximation of a self-oscillatory reaction system using the Laplace-Borel transform," Chaos, Solitons & Fractals, Elsevier, vol. 142(C).
  • Handle: RePEc:eee:chsofr:v:142:y:2021:i:c:s0960077920309000
    DOI: 10.1016/j.chaos.2020.110508
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