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Fabrication of robust and cost-efficient Hoffmann-type MOF sensors for room temperature ammonia detection

Author

Listed:
  • Sa Wang

    (Nankai University
    Nankai University)

  • Yu Fu

    (Xi’an Jiaotong University)

  • Ting Wang

    (Nankai University
    Nankai University)

  • Wansheng Liu

    (Nankai University
    Nankai University)

  • Jian Wang

    (Nankai University
    Nankai University)

  • Peng Zhao

    (Nankai University)

  • Heping Ma

    (Xi’an Jiaotong University)

  • Yao Chen

    (Nankai University
    Nankai University)

  • Peng Cheng

    (Nankai University
    Nankai University
    Nankai University)

  • Zhenjie Zhang

    (Nankai University
    Nankai University
    Nankai University)

Abstract

The development of fast-response sensors for detecting NH3 at room temperature remains a formidable challenge. Here, to address this challenge, two highly robust Hoffmann-type metal-organic frameworks are rationally applied as the NH3 sensing materials which possess ultra-high static adsorption capacity for NH3, only lower than the current benchmark material. The adsorption mechanism is in-depth unveiled by dynamic adsorption and simulation studies. The assembled interdigital electrode device exhibits low detection limit (25 ppb) and short response time (5 s) at room temperature, which set a record among all electrical signal sensors. Moreover, the sensor exhibits excellent selectivity towards NH3 in the presence of 13 other potential interfering gases. Prominently, the sensor can stably output signals for more than two months at room temperature and can be recovered by simply purging nitrogen at room temperature without heating. This study opens up a way for reasonably designing gas sensing materials for toxic gases.

Suggested Citation

  • Sa Wang & Yu Fu & Ting Wang & Wansheng Liu & Jian Wang & Peng Zhao & Heping Ma & Yao Chen & Peng Cheng & Zhenjie Zhang, 2023. "Fabrication of robust and cost-efficient Hoffmann-type MOF sensors for room temperature ammonia detection," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-42959-z
    DOI: 10.1038/s41467-023-42959-z
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    References listed on IDEAS

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    1. M. R. Tchalala & P. M. Bhatt & K. N. Chappanda & S. R. Tavares & K. Adil & Y. Belmabkhout & A. Shkurenko & A. Cadiau & N. Heymans & G. Weireld & G. Maurin & K. N. Salama & M. Eddaoudi, 2019. "Fluorinated MOF platform for selective removal and sensing of SO2 from flue gas and air," Nature Communications, Nature, vol. 10(1), pages 1-10, December.
    2. Xin Zhang & Eric A. Davidson & Denise L. Mauzerall & Timothy D. Searchinger & Patrice Dumas & Ye Shen, 2015. "Managing nitrogen for sustainable development," Nature, Nature, vol. 528(7580), pages 51-59, December.
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