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Enhanced Electrochemical Performances of Hollow-Structured N-Doped Carbon Derived from a Zeolitic Imidazole Framework (ZIF-8) Coated by Polydopamine as an Anode for Lithium-Ion Batteries

Author

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  • Da-Won Lee

    (Department of Chemistry, Dong-A University, Busan 49315, Korea
    Department of Chemical Engineering (BK21 FOUR Graduate Program), Dong-A University, Busan 49315, Korea
    These authors contributed equally to this work.)

  • Achmad Yanuar Maulana

    (Department of Chemistry, Dong-A University, Busan 49315, Korea
    These authors contributed equally to this work.)

  • Chaeeun Lee

    (Department of Chemistry, Dong-A University, Busan 49315, Korea
    Department of Chemical Engineering (BK21 FOUR Graduate Program), Dong-A University, Busan 49315, Korea)

  • Jungwook Song

    (Department of Chemistry, Dong-A University, Busan 49315, Korea
    Department of Chemical Engineering (BK21 FOUR Graduate Program), Dong-A University, Busan 49315, Korea)

  • Cybelle M. Futalan

    (Department of Environmental Science, Ateneo de Manila University, Quezon City 1108, Philippines)

  • Jongsik Kim

    (Department of Chemistry, Dong-A University, Busan 49315, Korea
    Department of Chemical Engineering (BK21 FOUR Graduate Program), Dong-A University, Busan 49315, Korea)

Abstract

Doping heteroatoms such as nitrogen (N) and boron (B) into the framework of carbon materials is one of the most efficient methods to improve the electrical performance of carbon-based electrodes. In this study, N-doped carbon has been facilely synthesized using a ZIF-8/polydopamine precursor. The polyhedral structure of ZIF-8 and the effective surface-coating capability of dopamine enabled the formation of N-doped carbon with a hollow structure. The ZIF-8 polyhedron served as a sacrificial template for hollow structures, and dopamine participated as a donor of the nitrogen element. When compared to ZIF-8-derived carbon, the HSNC electrode showed an improved reversible capacity of approximately 1398 mAh·g −1 after 100 cycles, with excellent cycling retention at a voltage range of 0.01 to 3.0 V using a current density of 0.1 A·g −1 .

Suggested Citation

  • Da-Won Lee & Achmad Yanuar Maulana & Chaeeun Lee & Jungwook Song & Cybelle M. Futalan & Jongsik Kim, 2021. "Enhanced Electrochemical Performances of Hollow-Structured N-Doped Carbon Derived from a Zeolitic Imidazole Framework (ZIF-8) Coated by Polydopamine as an Anode for Lithium-Ion Batteries," Energies, MDPI, vol. 14(9), pages 1-12, April.
    • Handle: RePEc:gam:jeners:v:14:y:2021:i:9:p:2436-:d:542843
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    References listed on IDEAS

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    1. Arumugam Manthiram, 2020. "A reflection on lithium-ion battery cathode chemistry," Nature Communications, Nature, vol. 11(1), pages 1-9, December.
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