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Highly active Ni/Al2O3 catalyst for CO2 methanation by the decomposition of Ni-MOF@Al2O3 precursor via cold plasma

Author

Listed:
  • Yu, Jiahui
  • Feng, Bingge
  • Liu, Shuai
  • Mu, Xueliang
  • Lester, Edward
  • Wu, Tao

Abstract

In this work, a novel Ni/Al2O3-P catalyst for CO2 methanation was prepared via an oxygen plasma decomposition of the Ni-MOF@Al2O3 core–shell precursor. The obtained catalyst showed a higher Ni dispersion (26.5%) and contained less NiAl2O4 spinel when compared with the Ni/Al2O3 prepared by the traditional method. The Ni/Al2O3-P catalyst showed significantly enhanced efficiency toward CO2 methanation as compared with those catalysts with a similar nickel loading but are prepared using the traditional method. For example, the space time yield of methane (STYCH4) of the Ni/Al2O3-P catalyst was as high as 21103.6 mg∙gNi-1∙h−1 at 400 °C and GHSV as 12000 ml∙g−1∙h−1, which is 3.4 times higher than that of the reported catalyst (6190.5 mg∙gNi-1∙h−1) with a similar nickel loading under similar reaction conditions. Moreover, Density Functional Theory (DFT) studies together with the CO2-TPD results revealed that both nickel surface and Ni-Al2O3 interface could activate CO2, while the NiAl2O4 surface could not.

Suggested Citation

  • Yu, Jiahui & Feng, Bingge & Liu, Shuai & Mu, Xueliang & Lester, Edward & Wu, Tao, 2022. "Highly active Ni/Al2O3 catalyst for CO2 methanation by the decomposition of Ni-MOF@Al2O3 precursor via cold plasma," Applied Energy, Elsevier, vol. 315(C).
    • Handle: RePEc:eee:appene:v:315:y:2022:i:c:s0306261922004408
    DOI: 10.1016/j.apenergy.2022.119036
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    References listed on IDEAS

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    1. Wang, Xiaoliu & Yang, Meng & Zhu, Xiaonan & Zhu, Lingjun & Wang, Shurong, 2020. "Experimental study and life cycle assessment of CO2 methanation over biochar supported catalysts," Applied Energy, Elsevier, vol. 280(C).
    2. Uebbing, Jennifer & Rihko-Struckmann, Liisa K. & Sundmacher, Kai, 2019. "Exergetic assessment of CO2 methanation processes for the chemical storage of renewable energies," Applied Energy, Elsevier, vol. 233, pages 271-282.
    3. Stangeland, Kristian & Kalai, Dori Yosef & Li, Hailong & Yu, Zhixin, 2018. "Active and stable Ni based catalysts and processes for biogas upgrading: The effect of temperature and initial methane concentration on CO2 methanation," Applied Energy, Elsevier, vol. 227(C), pages 206-212.
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    1. Guo, Junyan & Gao, Ruihong & Tong, Zhaoming & Zhang, Haijun & Duan, Hongjuan & Huang, Liang & Lu, Lilin & Jia, Quanli & Zhang, Shaowei, 2023. "Three eagles with one arrow: Simultaneous production of hydrogen, aluminum ethoxide, and supported metal catalysts via efficient and facile reaction between aluminum and ethanol," Energy, Elsevier, vol. 263(PD).

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