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Simulation of elevated temperature solid sorbent CO2 capture for pre-combustion applications using computational fluid dynamics

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  • Chen, Qin
  • Rosner, Fabian
  • Rao, Ashok
  • Samuelsen, Scott
  • Jayaraman, Ambal
  • Alptekin, Gokhan

Abstract

CO2 adsorption is one of the warm gas cleanup technologies under development for integrated gasification combined cycle (IGCC) applications. Computational Fluid Dynamics (CFD) can be a practical and powerful tool for reactor design for and optimization of the CO2 adsorption process. In this present work, CFD simulation was developed in commercially available ANSYS Fluent software and validated for solid sorbent CO2 capture to investigate pressure swing adsorption (PSA) for CO2 separation from syngas with all the auxiliary operating steps. The adsorption equilibrium and kinetics were incorporated into ANSYS by user defined functions (UDFs) for source terms in Navier–Stokes equations. The CFD model well predicted the CO2 breakthrough curve and temperature change. It was shown that in demo reactor operation, at the end of adsorption step, only half of the sorbent was loaded with CO2, while most of the loaded CO2 was released during the desorption step. Further optimization of sorbent packing and cycle operation can be done with assistance of this CFD model to maximize bed loading, and used to design the commercial size reactors.

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  • Chen, Qin & Rosner, Fabian & Rao, Ashok & Samuelsen, Scott & Jayaraman, Ambal & Alptekin, Gokhan, 2019. "Simulation of elevated temperature solid sorbent CO2 capture for pre-combustion applications using computational fluid dynamics," Applied Energy, Elsevier, vol. 237(C), pages 314-325.
    • Handle: RePEc:eee:appene:v:237:y:2019:i:c:p:314-325
    DOI: 10.1016/j.apenergy.2019.01.042
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    References listed on IDEAS

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    1. Chen, Qin & Rao, Ashok & Samuelsen, Scott, 2015. "Coproduction of transportation fuels in advanced IGCCs via coal and biomass mixtures," Applied Energy, Elsevier, vol. 157(C), pages 851-860.
    2. Chen, Qin & Rao, Ashok & Samuelsen, Scott, 2014. "H2 coproduction in IGCC with CCS via coal and biomass mixture using advanced technologies," Applied Energy, Elsevier, vol. 118(C), pages 258-270.
    3. Hedin, Niklas & Andersson, Linnéa & Bergström, Lennart & Yan, Jinyue, 2013. "Adsorbents for the post-combustion capture of CO2 using rapid temperature swing or vacuum swing adsorption," Applied Energy, Elsevier, vol. 104(C), pages 418-433.
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    1. Chi, Changyun & Li, Yingjie & Zhang, Wan & Wang, Zeyan, 2019. "Synthesis of a hollow microtubular Ca/Al sorbent with high CO2 uptake by hard templating," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    2. Zhao, Haitao & Ezeh, Collins I. & Ren, Weijia & Li, Wentao & Pang, Cheng Heng & Zheng, Chenghang & Gao, Xiang & Wu, Tao, 2019. "Integration of machine learning approaches for accelerated discovery of transition-metal dichalcogenides as Hg0 sensing materials," Applied Energy, Elsevier, vol. 254(C).
    3. Rosner, Fabian & Chen, Qin & Rao, Ashok & Samuelsen, Scott, 2020. "Thermo-economic analyses of isothermal water gas shift reactor integrations into IGCC power plant," Applied Energy, Elsevier, vol. 277(C).
    4. Rosner, Fabian & Chen, Qin & Rao, Ashok & Samuelsen, Scott & Jayaraman, Ambal & Alptekin, Gokhan, 2019. "Thermo-economic analyses of IGCC power plants employing warm gas CO2 separation technology," Energy, Elsevier, vol. 185(C), pages 541-553.
    5. Chen, Qin & Rosner, Fabian & Rao, Ashok & Samuelsen, Scott & Bonnema, Michael & Jayaraman, Ambal & Alptekin, Gokhan, 2020. "Simulation of elevated temperature combined water gas shift and solid sorbent CO2 capture for pre-combustion applications using computational fluid dynamics," Applied Energy, Elsevier, vol. 267(C).
    6. Yang, Shiliang & Zhou, Tao & Wei, Yonggang & Hu, Jianhang & Wang, Hua, 2020. "Dynamical and thermal property of rising bubbles in the bubbling fluidized biomass gasifier with wide particle size distribution," Applied Energy, Elsevier, vol. 259(C).
    7. Pashchenko, Dmitry, 2023. "Hydrogen-rich gas as a fuel for the gas turbines: A pathway to lower CO2 emission," Renewable and Sustainable Energy Reviews, Elsevier, vol. 173(C).
    8. Subraveti, Sai Gokul & Pai, Kasturi Nagesh & Rajagopalan, Ashwin Kumar & Wilkins, Nicholas Stiles & Rajendran, Arvind & Jayaraman, Ambalavan & Alptekin, Gokhan, 2019. "Cycle design and optimization of pressure swing adsorption cycles for pre-combustion CO2 capture," Applied Energy, Elsevier, vol. 254(C).

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