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Renewable diesel blendstocks produced by hydrothermal liquefaction of wet biowaste

Author

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  • Wan-Ting Chen

    (University of Illinois at Urbana-Champaign)

  • Yuanhui Zhang

    (University of Illinois at Urbana-Champaign
    China Agricultural University)

  • Timothy H. Lee

    (University of Illinois at Urbana-Champaign)

  • Zhenwei Wu

    (University of Illinois at Urbana-Champaign)

  • Buchun Si

    (University of Illinois at Urbana-Champaign
    China Agricultural University)

  • Chia-Fon F. Lee

    (University of Illinois at Urbana-Champaign)

  • Alice Lin

    (University of Illinois at Urbana-Champaign)

  • Brajendra K. Sharma

    (University of Illinois at Urbana-Champaign)

Abstract

Processing wet biowaste to create a useful product, a practice called valorization, is environmentally sustainable and has the potential to augment energy production. Biocrude converted from wet biowaste using hydrothermal liquefaction (HTL) has comparable heating values to petroleum crude. However, its composition is too complex for use as transportation fuels. Here, we show that distillation combined with esterification can effectively upgrade HTL biocrude oil into diesel blendstock. We demonstrate that the HTL biocrude oil converted from food processing waste and animal manure can be distilled into fractions with similar energy content to that of petroleum diesel. We then reduce the acidity of distillates through esterification to meet the diesel standard. Engine tests performed using 10–20% upgraded distillates blended with diesel show 96–100% power output, 101–102% NOx, 89–91% CO, 92–125% unburned hydrocarbon and 109–115% soot emissions, compared with regular diesel. HTL integrated with distillation and esterification has a higher energy recovery ratio than anaerobic digestion, lipid extraction, HTL combined with hydrotreating and producing diesel from petroleum. This approach realizes the potential of wet biowaste to alleviate petroleum consumption and to reduce greenhouse gas emissions.

Suggested Citation

  • Wan-Ting Chen & Yuanhui Zhang & Timothy H. Lee & Zhenwei Wu & Buchun Si & Chia-Fon F. Lee & Alice Lin & Brajendra K. Sharma, 2018. "Renewable diesel blendstocks produced by hydrothermal liquefaction of wet biowaste," Nature Sustainability, Nature, vol. 1(11), pages 702-710, November.
  • Handle: RePEc:nat:natsus:v:1:y:2018:i:11:d:10.1038_s41893-018-0172-3
    DOI: 10.1038/s41893-018-0172-3
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    Cited by:

    1. Shijie Yu & Xinyue Dong & Peng Zhao & Zhicheng Luo & Zhuohua Sun & Xiaoxiao Yang & Qinghai Li & Lei Wang & Yanguo Zhang & Hui Zhou, 2022. "Decoupled temperature and pressure hydrothermal synthesis of carbon sub-micron spheres from cellulose," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    2. Shahbeik, Hossein & Kazemi Shariat Panahi, Hamed & Dehhaghi, Mona & Guillemin, Gilles J. & Fallahi, Alireza & Hosseinzadeh-Bandbafha, Homa & Amiri, Hamid & Rehan, Mohammad & Raikwar, Deepak & Latine, , 2024. "Biomass to biofuels using hydrothermal liquefaction: A comprehensive review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 189(PB).
    3. Si, Buchun & Watson, Jamison & Wang, Zixin & Wang, Tengfei & Acero Triana, Juan S. & Zhang, Yuanhui, 2024. "Storage stability of biocrude oil fractional distillates derived from the hydrothermal liquefaction of food waste," Renewable Energy, Elsevier, vol. 220(C).
    4. Komeil Kohansal & Kamaldeep Sharma & Saqib Sohail Toor & Eliana Lozano Sanchez & Joscha Zimmermann & Lasse Aistrup Rosendahl & Thomas Helmer Pedersen, 2021. "Bio-Crude Production Improvement during Hydrothermal Liquefaction of Biopulp by Simultaneous Application of Alkali Catalysts and Aqueous Phase Recirculation," Energies, MDPI, vol. 14(15), pages 1-21, July.
    5. Huang, Yingying & Chen, Xuechu & Liu, Silu & Lu, Jinzhong & Shen, Yingshi & Li, Lei & Peng, Lin & Hong, Jingjie & Zhang, Qiuzhuo & Ostrovsky, Ilia, 2021. "Converting of nuisance cyanobacterial biomass to feedstock for bioethanol production by regulation of intracellular carbon flow: Killing two birds with one stone," Renewable and Sustainable Energy Reviews, Elsevier, vol. 149(C).
    6. Krogh, Andreas & Lozano, Eliana M. & Grue, Jeppe & Pedersen, Thomas H., 2024. "Assessment of feasible site locations for biofuel production based on technoeconomic modelling and GHG impact analysis," Applied Energy, Elsevier, vol. 356(C).

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