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Effect of support material on the performance of K2CO3-based pellets for cyclic CO2 capture

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  • Qin, Changlei
  • Yin, Junjun
  • Ran, Jingyu
  • Zhang, Li
  • Feng, Bo

Abstract

The K2CO3-based sorbent is promising for CO2 capture from the flue gas of fossil-fuel-fired power plant. In this work, various support/binder materials were utilized to prepare K2CO3-based sorbent pellets by an extrusion method, and their mechanical strength and CO2 capture performance were studied with different techniques. Results show that both the type of support/binder used and the content of K2CO3 have significant impact on the performance of the sorbents for CO2 capture. Among the sorbents prepared, K2CO3/Al2O3 exhibited the highest CO2 capture capacity of 71mg-CO2/g-sorbent, while K2CO3/clay demonstrated a much better compressive strength (25.2MPa), resistance to attrition and an interesting phenomenon of increased CO2 capture capacity with the number of cycles. It was also found that the support/binder material affects the physical properties of the pellets significantly.

Suggested Citation

  • Qin, Changlei & Yin, Junjun & Ran, Jingyu & Zhang, Li & Feng, Bo, 2014. "Effect of support material on the performance of K2CO3-based pellets for cyclic CO2 capture," Applied Energy, Elsevier, vol. 136(C), pages 280-288.
    • Handle: RePEc:eee:appene:v:136:y:2014:i:c:p:280-288
    DOI: 10.1016/j.apenergy.2014.09.043
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    References listed on IDEAS

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    Cited by:

    1. Jayakumar, Abhimanyu & Gomez, Arturo & Mahinpey, Nader, 2016. "Post-combustion CO2 capture using solid K2CO3: Discovering the carbonation reaction mechanism," Applied Energy, Elsevier, vol. 179(C), pages 531-543.
    2. Thummakul, Theeranan & Gidaspow, Dimitri & Piumsomboon, Pornpote & Chalermsinsuwan, Benjapon, 2017. "CFD simulation of CO2 sorption on K2CO3 solid sorbent in novel high flux circulating-turbulent fluidized bed riser: Parametric statistical experimental design study," Applied Energy, Elsevier, vol. 190(C), pages 122-134.
    3. Jiaquan Li & Yunbing Hou & Pengtao Wang & Bo Yang, 2018. "A Review of Carbon Capture and Storage Project Investment and Operational Decision-Making Based on Bibliometrics," Energies, MDPI, vol. 12(1), pages 1-22, December.
    4. Kong, Yong & Shen, Xiaodong & Cui, Sheng & Fan, Maohong, 2015. "Development of monolithic adsorbent via polymeric sol–gel process for low-concentration CO2 capture," Applied Energy, Elsevier, vol. 147(C), pages 308-317.
    5. Ju, Youngsan & Lee, Chang-Ha, 2019. "Dynamic modeling of a dual fluidized-bed system with the circulation of dry sorbent for CO2 capture," Applied Energy, Elsevier, vol. 241(C), pages 640-651.

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    Keywords

    K2CO3-based sorbents; CO2 capture; Sorbent pellets;
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