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Two-dimensional semiconducting SnP2Se6 with giant second-harmonic-generation for monolithic on-chip electronic-photonic integration

Author

Listed:
  • Cheng-Yi Zhu

    (Harbin Institute of Technology (Shenzhen))

  • Zimeng Zhang

    (Harbin Institute of Technology (Shenzhen))

  • Jing-Kai Qin

    (Harbin Institute of Technology (Shenzhen))

  • Zi Wang

    (Harbin Institute of Technology (Shenzhen))

  • Cong Wang

    (The Hong Kong Polytechnic University)

  • Peng Miao

    (HORIBA Scientific)

  • Yingjie Liu

    (Harbin Institute of Technology (Shenzhen))

  • Pei-Yu Huang

    (Harbin Institute of Technology (Shenzhen))

  • Yao Zhang

    (Harbin Institute of Technology (Shenzhen))

  • Ke Xu

    (Harbin Institute of Technology (Shenzhen))

  • Liang Zhen

    (Harbin Institute of Technology (Shenzhen)
    Harbin Institute of Technology)

  • Yang Chai

    (The Hong Kong Polytechnic University)

  • Cheng-Yan Xu

    (Harbin Institute of Technology (Shenzhen)
    Harbin Institute of Technology)

Abstract

Two-dimensional (2D) layered semiconductors with nonlinear optical (NLO) properties hold great promise to address the growing demand of multifunction integration in electronic-photonic integrated circuits (EPICs). However, electronic-photonic co-design with 2D NLO semiconductors for on-chip telecommunication is limited by their essential shortcomings in terms of unsatisfactory optoelectronic properties, odd-even layer-dependent NLO activity and low NLO susceptibility in telecom band. Here we report the synthesis of 2D SnP2Se6, a van der Waals NLO semiconductor exhibiting strong odd-even layer-independent second harmonic generation (SHG) activity at 1550 nm and pronounced photosensitivity under visible light. The combination of 2D SnP2Se6 with a SiN photonic platform enables the chip-level multifunction integration for EPICs. The hybrid device not only features efficient on-chip SHG process for optical modulation, but also allows the telecom-band photodetection relying on the upconversion of wavelength from 1560 to 780 nm. Our finding offers alternative opportunities for the collaborative design of EPICs.

Suggested Citation

  • Cheng-Yi Zhu & Zimeng Zhang & Jing-Kai Qin & Zi Wang & Cong Wang & Peng Miao & Yingjie Liu & Pei-Yu Huang & Yao Zhang & Ke Xu & Liang Zhen & Yang Chai & Cheng-Yan Xu, 2023. "Two-dimensional semiconducting SnP2Se6 with giant second-harmonic-generation for monolithic on-chip electronic-photonic integration," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-38131-2
    DOI: 10.1038/s41467-023-38131-2
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