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Room-temperature polariton quantum fluids in halide perovskites

Author

Listed:
  • Kai Peng

    (University of Nebraska-Lincoln)

  • Renjie Tao

    (University of California)

  • Louis Haeberlé

    (École Polytechnique de Montréal)

  • Quanwei Li

    (University of California)

  • Dafei Jin

    (Argonne National Laboratory)

  • Graham R. Fleming

    (University of California)

  • Stéphane Kéna-Cohen

    (École Polytechnique de Montréal)

  • Xiang Zhang

    (University of California
    The University of Hong Kong)

  • Wei Bao

    (University of Nebraska-Lincoln)

Abstract

Quantum fluids exhibit quantum mechanical effects at the macroscopic level, which contrast strongly with classical fluids. Gain-dissipative solid-state exciton-polaritons systems are promising emulation platforms for complex quantum fluid studies at elevated temperatures. Recently, halide perovskite polariton systems have emerged as materials with distinctive advantages over other room-temperature systems for future studies of topological physics, non-Abelian gauge fields, and spin-orbit interactions. However, the demonstration of nonlinear quantum hydrodynamics, such as superfluidity and Čerenkov flow, which is a consequence of the renormalized elementary excitation spectrum, remains elusive in halide perovskites. Here, using homogenous halide perovskites single crystals, we report, in both one- and two-dimensional cases, the complete set of quantum fluid phase transitions from normal classical fluids to scatterless polariton superfluids and supersonic fluids—all at room temperature, clear consequences of the Landau criterion. Specifically, the supersonic Čerenkov wave pattern was observed at room temperature. The experimental results are also in quantitative agreement with theoretical predictions from the dissipative Gross-Pitaevskii equation. Our results set the stage for exploring the rich non-equilibrium quantum fluid many-body physics at room temperature and also pave the way for important polaritonic device applications.

Suggested Citation

  • Kai Peng & Renjie Tao & Louis Haeberlé & Quanwei Li & Dafei Jin & Graham R. Fleming & Stéphane Kéna-Cohen & Xiang Zhang & Wei Bao, 2022. "Room-temperature polariton quantum fluids in halide perovskites," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-34987-y
    DOI: 10.1038/s41467-022-34987-y
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    References listed on IDEAS

    as
    1. Yao Li & Xuekai Ma & Xiaokun Zhai & Meini Gao & Haitao Dai & Stefan Schumacher & Tingge Gao, 2022. "Author Correction: Manipulating polariton condensates by Rashba-Dresselhaus coupling at room temperature," Nature Communications, Nature, vol. 13(1), pages 1-1, December.
    2. Haotong Wei & Jinsong Huang, 2019. "Halide lead perovskites for ionizing radiation detection," Nature Communications, Nature, vol. 10(1), pages 1-12, December.
    3. Maciej Pieczarka & Eliezer Estrecho & Maryam Boozarjmehr & Olivier Bleu & Mark Steger & Kenneth West & Loren N. Pfeiffer & David W. Snoke & Jesper Levinsen & Meera M. Parish & Andrew G. Truscott & Ele, 2020. "Observation of quantum depletion in a non-equilibrium exciton–polariton condensate," Nature Communications, Nature, vol. 11(1), pages 1-7, December.
    4. R. T. Juggins & J. Keeling & M. H. Szymańska, 2018. "Coherently driven microcavity-polaritons and the question of superfluidity," Nature Communications, Nature, vol. 9(1), pages 1-8, December.
    5. J. -M. Ménard & C. Poellmann & M. Porer & U. Leierseder & E. Galopin & A. Lemaître & A. Amo & J. Bloch & R. Huber, 2014. "Revealing the dark side of a bright exciton–polariton condensate," Nature Communications, Nature, vol. 5(1), pages 1-5, December.
    6. A. Gianfrate & O. Bleu & L. Dominici & V. Ardizzone & M. Giorgi & D. Ballarini & G. Lerario & K. W. West & L. N. Pfeiffer & D. D. Solnyshkov & D. Sanvitto & G. Malpuech, 2020. "Measurement of the quantum geometric tensor and of the anomalous Hall drift," Nature, Nature, vol. 578(7795), pages 381-385, February.
    7. Petr Stepanov & Ivan Amelio & Jean-Guy Rousset & Jacqueline Bloch & Aristide Lemaître & Alberto Amo & Anna Minguzzi & Iacopo Carusotto & Maxime Richard, 2019. "Dispersion relation of the collective excitations in a resonantly driven polariton fluid," Nature Communications, Nature, vol. 10(1), pages 1-8, December.
    8. Yao Li & Xuekai Ma & Xiaokun Zhai & Meini Gao & Haitao Dai & Stefan Schumacher & Tingge Gao, 2022. "Manipulating polariton condensates by Rashba-Dresselhaus coupling at room temperature," Nature Communications, Nature, vol. 13(1), pages 1-6, December.
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