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Annual cycle observations of aerosols capable of ice formation in central Arctic clouds

Author

Listed:
  • Jessie M. Creamean

    (Colorado State University)

  • Kevin Barry

    (Colorado State University)

  • Thomas C. J. Hill

    (Colorado State University)

  • Carson Hume

    (Colorado State University)

  • Paul J. DeMott

    (Colorado State University)

  • Matthew D. Shupe

    (University of Colorado
    Physical Sciences Laboratory, National Oceanic and Atmospheric Administration)

  • Sandro Dahlke

    (Climate Sciences Division, Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung)

  • Sascha Willmes

    (Universität Trier)

  • Julia Schmale

    (Extreme Environments Research Laboratory, École Polytechnique Fédérale de Lausanne)

  • Ivo Beck

    (Extreme Environments Research Laboratory, École Polytechnique Fédérale de Lausanne)

  • Clara J. M. Hoppe

    (Biosciences Division, Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung)

  • Allison Fong

    (Biosciences Division, Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung)

  • Emelia Chamberlain

    (University of California)

  • Jeff Bowman

    (University of California)

  • Randall Scharien

    (University of Victoria)

  • Ola Persson

    (University of Colorado
    Physical Sciences Laboratory, National Oceanic and Atmospheric Administration)

Abstract

The Arctic is warming faster than anywhere else on Earth, prompting glacial melt, permafrost thaw, and sea ice decline. These severe consequences induce feedbacks that contribute to amplified warming, affecting weather and climate globally. Aerosols and clouds play a critical role in regulating radiation reaching the Arctic surface. However, the magnitude of their effects is not adequately quantified, especially in the central Arctic where they impact the energy balance over the sea ice. Specifically, aerosols called ice nucleating particles (INPs) remain understudied yet are necessary for cloud ice production and subsequent changes in cloud lifetime, radiative effects, and precipitation. Here, we report observations of INPs in the central Arctic over a full year, spanning the entire sea ice growth and decline cycle. Further, these observations are size-resolved, affording valuable information on INP sources. Our results reveal a strong seasonality of INPs, with lower concentrations in the winter and spring controlled by transport from lower latitudes, to enhanced concentrations of INPs during the summer melt, likely from marine biological production in local open waters. This comprehensive characterization of INPs will ultimately help inform cloud parameterizations in models of all scales.

Suggested Citation

  • Jessie M. Creamean & Kevin Barry & Thomas C. J. Hill & Carson Hume & Paul J. DeMott & Matthew D. Shupe & Sandro Dahlke & Sascha Willmes & Julia Schmale & Ivo Beck & Clara J. M. Hoppe & Allison Fong & , 2022. "Annual cycle observations of aerosols capable of ice formation in central Arctic clouds," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-31182-x
    DOI: 10.1038/s41467-022-31182-x
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    References listed on IDEAS

    as
    1. Andrea Baccarini & Linn Karlsson & Josef Dommen & Patrick Duplessis & Jutta Vüllers & Ian M. Brooks & Alfonso Saiz-Lopez & Matthew Salter & Michael Tjernström & Urs Baltensperger & Paul Zieger & Julia, 2020. "Frequent new particle formation over the high Arctic pack ice by enhanced iodine emissions," Nature Communications, Nature, vol. 11(1), pages 1-11, December.
    2. Andrea Baccarini & Linn Karlsson & Josef Dommen & Patrick Duplessis & Jutta Vüllers & Ian M. Brooks & Alfonso Saiz-Lopez & Matthew Salter & Michael Tjernström & Urs Baltensperger & Paul Zieger & Julia, 2020. "Publisher Correction: Frequent new particle formation over the high Arctic pack ice by enhanced iodine emissions," Nature Communications, Nature, vol. 11(1), pages 1-1, December.
    3. Theodore W. Wilson & Luis A. Ladino & Peter A. Alpert & Mark N. Breckels & Ian M. Brooks & Jo Browse & Susannah M. Burrows & Kenneth S. Carslaw & J. Alex Huffman & Christopher Judd & Wendy P. Kilthau , 2015. "A marine biogenic source of atmospheric ice-nucleating particles," Nature, Nature, vol. 525(7568), pages 234-238, September.
    4. Julia Schmale & Paul Zieger & Annica M. L. Ekman, 2021. "Aerosols in current and future Arctic climate," Nature Climate Change, Nature, vol. 11(2), pages 95-105, February.
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    Cited by:

    1. Gabriel Pereira Freitas & Kouji Adachi & Franz Conen & Dominic Heslin-Rees & Radovan Krejci & Yutaka Tobo & Karl Espen Yttri & Paul Zieger, 2023. "Regionally sourced bioaerosols drive high-temperature ice nucleating particles in the Arctic," Nature Communications, Nature, vol. 14(1), pages 1-10, December.

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