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Influence Of The Reaction Temperature On The Oscillatory Behavior During Partial Oxidation Of Methane

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  • XIU-BIN REN

    (State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001, P. R. China;
    Graduate University of the Chinese Academy of Sciences, Beijing 100039, P. R. China)

  • XIANG-YUN GUO

    (State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001, P. R. China)

Abstract

The oscillatory behavior during partial oxidation of methane was studied by the Monte Carlo simulation with Langmuir–Hinshelwood mechanism and oxide formation and removal. The well-developed reaction rate oscillations can be observed when theCH4adsorption probability varies in a small window. The oscillation window is very sensitive to the variation of reaction temperature. When the temperature increases, the window for sustained oscillation becomes narrow and has an obvious shift. In the meantime, the oscillation period tends to become small and the amplitude decreases. When the temperature increases to a certain value, the oscillations will disappear.

Suggested Citation

  • Xiu-Bin Ren & Xiang-Yun Guo, 2008. "Influence Of The Reaction Temperature On The Oscillatory Behavior During Partial Oxidation Of Methane," Surface Review and Letters (SRL), World Scientific Publishing Co. Pte. Ltd., vol. 15(06), pages 769-774.
    • Handle: RePEc:wsi:srlxxx:v:15:y:2008:i:06:n:s0218625x0801213x
    DOI: 10.1142/S0218625X0801213X
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