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A New Approach Of The Sims Method For Metal Clusters

Author

Listed:
  • I. KATAKUSE

    (Department of Earth and Space Science, Faculty of Science, Osaka University, Machikaneyama-cho, Toyonaka, Osaka 560, Japan)

  • T. ICHIHARA

    (Department of Earth and Space Science, Faculty of Science, Osaka University, Machikaneyama-cho, Toyonaka, Osaka 560, Japan)

  • H. ITO

    (Department of Physics, Faculty of Science, Osaka University, Machikaneyama-cho, Toyonaka, Osaka 560, Japan)

  • T. SAKURAI

    (Department of Physics, Faculty of Science, Osaka University, Machikaneyama-cho, Toyonaka, Osaka 560, Japan)

  • T. MATSUO

    (Department of Physics, Faculty of Science, Osaka University, Machikaneyama-cho, Toyonaka, Osaka 560, Japan)

Abstract

The size distributions of(CsI)nCs+,$({\rm MgO})_n^+ ({\rm MgO})_n {\rm Mg}^+$, and$({\rm Hg})_n M_j^+$(M:alkali metal,j=1, 2, 3, 4, 5) clusters were obtained using secondary-ion mass spectrometry. The sizes of stable neutral clusters(CsI)nand(Hg)nclusters were determined from the mass spectra of cluster ions(CsI)nCs+and(Hg)nM+. The magic numbers of$({\rm Hg})_n {\rm K}_3^+$clusters were identical to those of van der Waals type clusters. It is believed that the shell closing cluster${\rm K}_3^+$is at the center of complex clusters$({\rm Hg})_n {\rm K}_3^+$. The$({\rm Hg})_n {\rm K}_4^+$clusters were believed to have electronic shell structures from the magic numbers.

Suggested Citation

  • I. Katakuse & T. Ichihara & H. Ito & T. Sakurai & T. Matsuo, 1996. "A New Approach Of The Sims Method For Metal Clusters," Surface Review and Letters (SRL), World Scientific Publishing Co. Pte. Ltd., vol. 3(01), pages 551-555.
    • Handle: RePEc:wsi:srlxxx:v:03:y:1996:i:01:n:s0218625x96001005
    DOI: 10.1142/S0218625X96001005
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