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Cascade of correlated electron states in the kagome superconductor CsV3Sb5

Author

Listed:
  • He Zhao

    (Boston College)

  • Hong Li

    (Boston College)

  • Brenden R. Ortiz

    (University of California Santa Barbara)

  • Samuel M. L. Teicher

    (University of California Santa Barbara)

  • Takamori Park

    (University of California Santa Barbara)

  • Mengxing Ye

    (University of California, Santa Barbara)

  • Ziqiang Wang

    (Boston College)

  • Leon Balents

    (University of California, Santa Barbara
    Canadian Institute for Advanced Research)

  • Stephen D. Wilson

    (University of California Santa Barbara)

  • Ilija Zeljkovic

    (Boston College)

Abstract

The kagome lattice of transition metal atoms provides an exciting platform to study electronic correlations in the presence of geometric frustration and nontrivial band topology1–18, which continues to bear surprises. Here, using spectroscopic imaging scanning tunnelling microscopy, we discover a temperature-dependent cascade of different symmetry-broken electronic states in a new kagome superconductor, CsV3Sb5. We reveal, at a temperature far above the superconducting transition temperature Tc ~ 2.5 K, a tri-directional charge order with a 2a0 period that breaks the translation symmetry of the lattice. As the system is cooled down towards Tc, we observe a prominent V-shaped spectral gap opening at the Fermi level and an additional breaking of the six-fold rotational symmetry, which persists through the superconducting transition. This rotational symmetry breaking is observed as the emergence of an additional 4a0 unidirectional charge order and strongly anisotropic scattering in differential conductance maps. The latter can be directly attributed to the orbital-selective renormalization of the vanadium kagome bands. Our experiments reveal a complex landscape of electronic states that can coexist on a kagome lattice, and highlight intriguing parallels to high-Tc superconductors and twisted bilayer graphene.

Suggested Citation

  • He Zhao & Hong Li & Brenden R. Ortiz & Samuel M. L. Teicher & Takamori Park & Mengxing Ye & Ziqiang Wang & Leon Balents & Stephen D. Wilson & Ilija Zeljkovic, 2021. "Cascade of correlated electron states in the kagome superconductor CsV3Sb5," Nature, Nature, vol. 599(7884), pages 216-221, November.
  • Handle: RePEc:nat:nature:v:599:y:2021:i:7884:d:10.1038_s41586-021-03946-w
    DOI: 10.1038/s41586-021-03946-w
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    Cited by:

    1. Zhicheng Jiang & Zhengtai Liu & Haiyang Ma & Wei Xia & Zhonghao Liu & Jishan Liu & Soohyun Cho & Yichen Yang & Jianyang Ding & Jiayu Liu & Zhe Huang & Yuxi Qiao & Jiajia Shen & Wenchuan Jing & Xiangqi, 2023. "Flat bands, non-trivial band topology and rotation symmetry breaking in layered kagome-lattice RbTi3Bi5," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    2. M. Roppongi & K. Ishihara & Y. Tanaka & K. Ogawa & K. Okada & S. Liu & K. Mukasa & Y. Mizukami & Y. Uwatoko & R. Grasset & M. Konczykowski & B. R. Ortiz & S. D. Wilson & K. Hashimoto & T. Shibauchi, 2023. "Bulk evidence of anisotropic s-wave pairing with no sign change in the kagome superconductor CsV3Sb5," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    3. Yong Hu & Junzhang Ma & Yinxiang Li & Yuxiao Jiang & Dariusz Jakub Gawryluk & Tianchen Hu & Jérémie Teyssier & Volodymyr Multian & Zhouyi Yin & Shuxiang Xu & Soohyeon Shin & Igor Plokhikh & Xinloong H, 2024. "Phonon promoted charge density wave in topological kagome metal ScV6Sn6," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    4. Harley D. Scammell & Julian Ingham & Tommy Li & Oleg P. Sushkov, 2023. "Chiral excitonic order from twofold van Hove singularities in kagome metals," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    5. D. Subires & A. Korshunov & A. H. Said & L. Sánchez & Brenden R. Ortiz & Stephen D. Wilson & A. Bosak & S. Blanco-Canosa, 2023. "Order-disorder charge density wave instability in the kagome metal (Cs,Rb)V3Sb5," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    6. A. Korshunov & H. Hu & D. Subires & Y. Jiang & D. Călugăru & X. Feng & A. Rajapitamahuni & C. Yi & S. Roychowdhury & M. G. Vergniory & J. Strempfer & C. Shekhar & E. Vescovo & D. Chernyshov & A. H. Sa, 2023. "Softening of a flat phonon mode in the kagome ScV6Sn6," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    7. Camron Farhang & Jingyuan Wang & Brenden R. Ortiz & Stephen D. Wilson & Jing Xia, 2023. "Unconventional specular optical rotation in the charge ordered state of Kagome metal CsV3Sb5," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    8. Jiangang Yang & Xinwei Yi & Zhen Zhao & Yuyang Xie & Taimin Miao & Hailan Luo & Hao Chen & Bo Liang & Wenpei Zhu & Yuhan Ye & Jing-Yang You & Bo Gu & Shenjin Zhang & Fengfeng Zhang & Feng Yang & Zhimi, 2023. "Observation of flat band, Dirac nodal lines and topological surface states in Kagome superconductor CsTi3Bi5," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    9. Hui Chen & Yuqing Xing & Hengxin Tan & Li Huang & Qi Zheng & Zihao Huang & Xianghe Han & Bin Hu & Yuhan Ye & Yan Li & Yao Xiao & Hechang Lei & Xianggang Qiu & Enke Liu & Haitao Yang & Ziqiang Wang & B, 2024. "Atomically precise engineering of spin–orbit polarons in a kagome magnetic Weyl semimetal," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    10. Gan Liu & Xinran Ma & Kuanyu He & Qing Li & Hengxin Tan & Yizhou Liu & Jie Xu & Wenna Tang & Kenji Watanabe & Takashi Taniguchi & Libo Gao & Yaomin Dai & Hai-Hu Wen & Binghai Yan & Xiaoxiang Xi, 2022. "Observation of anomalous amplitude modes in the kagome metal CsV3Sb5," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    11. Yang Luo & Yulei Han & Jinjin Liu & Hui Chen & Zihao Huang & Linwei Huai & Hongyu Li & Bingqian Wang & Jianchang Shen & Shuhan Ding & Zeyu Li & Shuting Peng & Zhiyuan Wei & Yu Miao & Xiupeng Sun & Zhi, 2023. "A unique van Hove singularity in kagome superconductor CsV3-xTaxSb5 with enhanced superconductivity," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    12. Boqin Song & Tianping Ying & Xianxin Wu & Wei Xia & Qiangwei Yin & Qinghua Zhang & Yanpeng Song & Xiaofan Yang & Jiangang Guo & Lin Gu & Xiaolong Chen & Jiangping Hu & Andreas P. Schnyder & Hechang Le, 2023. "Anomalous enhancement of charge density wave in kagome superconductor CsV3Sb5 approaching the 2D limit," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    13. Ruoting Yin & Xiang Zhu & Qiang Fu & Tianyi Hu & Lingyun Wan & Yingying Wu & Yifan Liang & Zhengya Wang & Zhen-Lin Qiu & Yuan-Zhi Tan & Chuanxu Ma & Shijing Tan & Wei Hu & Bin Li & Z. F. Wang & Jinlon, 2024. "Artificial kagome lattices of Shockley surface states patterned by halogen hydrogen-bonded organic frameworks," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    14. Ge He & Leander Peis & Emma Frances Cuddy & Zhen Zhao & Dong Li & Yuhang Zhang & Romona Stumberger & Brian Moritz & Haitao Yang & Hongjun Gao & Thomas Peter Devereaux & Rudi Hackl, 2024. "Anharmonic strong-coupling effects at the origin of the charge density wave in CsV3Sb5," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    15. Sen Zhou & Ziqiang Wang, 2022. "Chern Fermi pocket, topological pair density wave, and charge-4e and charge-6e superconductivity in kagomé superconductors," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    16. Huimin Zhang & Basu Dev Oli & Qiang Zou & Xu Guo & Zhengfei Wang & Lian Li, 2023. "Visualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    17. Li Huang & Xianghua Kong & Qi Zheng & Yuqing Xing & Hui Chen & Yan Li & Zhixin Hu & Shiyu Zhu & Jingsi Qiao & Yu-Yang Zhang & Haixia Cheng & Zhihai Cheng & Xianggang Qiu & Enke Liu & Hechang Lei & Xia, 2023. "Discovery and construction of surface kagome electronic states induced by p-d electronic hybridization in Co3Sn2S2," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    18. H. Miao & T. T. Zhang & H. X. Li & G. Fabbris & A. H. Said & R. Tartaglia & T. Yilmaz & E. Vescovo & J.-X. Yin & S. Murakami & X. L. Feng & K. Jiang & X. L. Wu & A. F. Wang & S. Okamoto & Y. L. Wang &, 2023. "Signature of spin-phonon coupling driven charge density wave in a kagome magnet," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

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