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Unlocking full and fast conversion in photocatalytic carbon dioxide reduction for applications in radio-carbonylation

Author

Listed:
  • Serena Monticelli

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Alex Talbot

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Philipp Gotico

    (Université Paris-Saclay, CEA, CNRS, Institute for Integrative Biology of the Cell)

  • Fabien Caillé

    (Université Paris-Saclay, Inserm, CNRS, CEA, Laboratoire d’Imagerie Biomédicale Multimodale Paris-Saclay (BioMaps))

  • Olivier Loreau

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Antonio Vecchio

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Augustin Malandain

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Antoine Sallustrau

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Winfried Leibl

    (Université Paris-Saclay, CEA, CNRS, Institute for Integrative Biology of the Cell)

  • Ally Aukauloo

    (Université Paris-Saclay, CEA, CNRS, Institute for Integrative Biology of the Cell
    Université Paris-Saclay, CNRS, Institut de chimie moléculaire et des matériaux d’Orsay)

  • Frédéric Taran

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

  • Zakaria Halime

    (Université Paris-Saclay, CNRS, Institut de chimie moléculaire et des matériaux d’Orsay)

  • Davide Audisio

    (Université Paris-Saclay, CEA, Service de Chimie Bio-organique et Marquage, DMTS)

Abstract

Harvesting sunlight to drive carbon dioxide (CO2) valorisation represents an ideal concept to support a sustainable and carbon-neutral economy. While the photochemical reduction of CO2 to carbon monoxide (CO) has emerged as a hot research topic, the full CO2-to-CO conversion remains an often-overlooked criterion that prevents a productive and direct valorisation of CO into high-value-added chemicals. Herein, we report a photocatalytic process that unlocks full and fast CO2-to-CO conversion (

Suggested Citation

  • Serena Monticelli & Alex Talbot & Philipp Gotico & Fabien Caillé & Olivier Loreau & Antonio Vecchio & Augustin Malandain & Antoine Sallustrau & Winfried Leibl & Ally Aukauloo & Frédéric Taran & Zakari, 2023. "Unlocking full and fast conversion in photocatalytic carbon dioxide reduction for applications in radio-carbonylation," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-40136-w
    DOI: 10.1038/s41467-023-40136-w
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    References listed on IDEAS

    as
    1. Yuan-Sheng Xia & Meizhong Tang & Lei Zhang & Jiang Liu & Cheng Jiang & Guang-Kuo Gao & Long-Zhang Dong & Lan-Gui Xie & Ya-Qian Lan, 2022. "Tandem utilization of CO2 photoreduction products for the carbonylation of aryl iodides," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    2. Zutao Ouyang & Pietro Sciusco & Tong Jiao & Sarah Feron & Cheyenne Lei & Fei Li & Ranjeet John & Peilei Fan & Xia Li & Christopher A. Williams & Guangzhao Chen & Chenghao Wang & Jiquan Chen, 2022. "Albedo changes caused by future urbanization contribute to global warming," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    3. Rui Sang & Yuya Hu & Rauf Razzaq & Guillaume Mollaert & Hanan Atia & Ursula Bentrup & Muhammad Sharif & Helfried Neumann & Henrik Junge & Ralf Jackstell & Bert U. W. Maes & Matthias Beller, 2022. "A practical concept for catalytic carbonylations using carbon dioxide," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
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