IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v13y2022i1d10.1038_s41467-022-33016-2.html
   My bibliography  Save this article

Wide field imaging of van der Waals ferromagnet Fe3GeTe2 by spin defects in hexagonal boron nitride

Author

Listed:
  • Mengqi Huang

    (University of California, San Diego)

  • Jingcheng Zhou

    (University of California, San Diego)

  • Di Chen

    (University of Houston
    University of Houston)

  • Hanyi Lu

    (University of California, San Diego)

  • Nathan J. McLaughlin

    (University of California, San Diego)

  • Senlei Li

    (University of California, San Diego)

  • Mohammed Alghamdi

    (University of California)

  • Dziga Djugba

    (University of California, San Diego)

  • Jing Shi

    (University of California)

  • Hailong Wang

    (University of California, San Diego)

  • Chunhui Rita Du

    (University of California, San Diego
    University of California, San Diego)

Abstract

Emergent color centers with accessible spins hosted by van der Waals materials have attracted substantial interest in recent years due to their significant potential for implementing transformative quantum sensing technologies. Hexagonal boron nitride (hBN) is naturally relevant in this context due to its remarkable ease of integration into devices consisting of low-dimensional materials. Taking advantage of boron vacancy spin defects in hBN, we report nanoscale quantum imaging of low-dimensional ferromagnetism sustained in Fe3GeTe2/hBN van der Waals heterostructures. Exploiting spin relaxometry methods, we have further observed spatially varying magnetic fluctuations in the exfoliated Fe3GeTe2 flake, whose magnitude reaches a peak value around the Curie temperature. Our results demonstrate the capability of spin defects in hBN of investigating local magnetic properties of layered materials in an accessible and precise way, which can be extended readily to a broad range of miniaturized van der Waals heterostructure systems.

Suggested Citation

  • Mengqi Huang & Jingcheng Zhou & Di Chen & Hanyi Lu & Nathan J. McLaughlin & Senlei Li & Mohammed Alghamdi & Dziga Djugba & Jing Shi & Hailong Wang & Chunhui Rita Du, 2022. "Wide field imaging of van der Waals ferromagnet Fe3GeTe2 by spin defects in hexagonal boron nitride," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-33016-2
    DOI: 10.1038/s41467-022-33016-2
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-022-33016-2
    File Function: Abstract
    Download Restriction: no
    File URL: https://libkey.io/10.1038/s41467-022-33016-2?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. William F. Koehl & Bob B. Buckley & F. Joseph Heremans & Greg Calusine & David D. Awschalom, 2011. "Room temperature coherent control of defect spin qubits in silicon carbide," Nature, Nature, vol. 479(7371), pages 84-87, November.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Mengqi Huang & Zeliang Sun & Gerald Yan & Hongchao Xie & Nishkarsh Agarwal & Gaihua Ye & Suk Hyun Sung & Hanyi Lu & Jingcheng Zhou & Shaohua Yan & Shangjie Tian & Hechang Lei & Robert Hovden & Rui He , 2023. "Revealing intrinsic domains and fluctuations of moiré magnetism by a wide-field quantum microscope," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    2. Ruotian Gong & Xinyi Du & Eli Janzen & Vincent Liu & Zhongyuan Liu & Guanghui He & Bingtian Ye & Tongcang Li & Norman Y. Yao & James H. Edgar & Erik A. Henriksen & Chong Zu, 2024. "Isotope engineering for spin defects in van der Waals materials," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    3. Andrew J. Ramsay & Reza Hekmati & Charlie J. Patrickson & Simon Baber & David R. M. Arvidsson-Shukur & Anthony J. Bennett & Isaac J. Luxmoore, 2023. "Coherence protection of spin qubits in hexagonal boron nitride," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    4. Roberto Rizzato & Martin Schalk & Stephan Mohr & Jens C. Hermann & Joachim P. Leibold & Fleming Bruckmaier & Giovanna Salvitti & Chenjiang Qian & Peirui Ji & Georgy V. Astakhov & Ulrich Kentsch & Manf, 2023. "Extending the coherence of spin defects in hBN enables advanced qubit control and quantum sensing," Nature Communications, Nature, vol. 14(1), pages 1-9, December.

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Cunzhi Zhang & Francois Gygi & Giulia Galli, 2023. "Engineering the formation of spin-defects from first principles," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    2. Hanfeng Wang & Matthew E. Trusheim & Laura Kim & Hamza Raniwala & Dirk R. Englund, 2023. "Field programmable spin arrays for scalable quantum repeaters," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    3. Łukasz Dusanowski & Cornelius Nawrath & Simone L. Portalupi & Michael Jetter & Tobias Huber & Sebastian Klembt & Peter Michler & Sven Höfling, 2022. "Optical charge injection and coherent control of a quantum-dot spin-qubit emitting at telecom wavelengths," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    4. Zhe Cheng & Jianbo Liang & Keisuke Kawamura & Hao Zhou & Hidetoshi Asamura & Hiroki Uratani & Janak Tiwari & Samuel Graham & Yutaka Ohno & Yasuyoshi Nagai & Tianli Feng & Naoteru Shigekawa & David G. , 2022. "High thermal conductivity in wafer-scale cubic silicon carbide crystals," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    5. J. M. Kitzman & J. R. Lane & C. Undershute & P. M. Harrington & N. R. Beysengulov & C. A. Mikolas & K. W. Murch & J. Pollanen, 2023. "Phononic bath engineering of a superconducting qubit," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    6. Ruotian Gong & Xinyi Du & Eli Janzen & Vincent Liu & Zhongyuan Liu & Guanghui He & Bingtian Ye & Tongcang Li & Norman Y. Yao & James H. Edgar & Erik A. Henriksen & Chong Zu, 2024. "Isotope engineering for spin defects in van der Waals materials," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    7. Elizabeth M. Y. Lee & Alvin Yu & Juan J. de Pablo & Giulia Galli, 2021. "Stability and molecular pathways to the formation of spin defects in silicon carbide," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    8. Ruotian Gong & Guanghui He & Xingyu Gao & Peng Ju & Zhongyuan Liu & Bingtian Ye & Erik A. Henriksen & Tongcang Li & Chong Zu, 2023. "Coherent dynamics of strongly interacting electronic spin defects in hexagonal boron nitride," Nature Communications, Nature, vol. 14(1), pages 1-10, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-33016-2. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.