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Recent Progress in the Use of Perovskites for Electrochemical, Photoelectrochemical, and Photovoltaic–Electrochemical CO 2 Reduction

Author

Listed:
  • Mina Ahmadi-Kashani

    (Chemical Engineering Department, University of Kashan, Kashan 8731753153, Iran)

  • Mahmoud Zendehdel

    (Kimia Solar Research Institute (K.S.R.I), Kimia Solar Company, Kashan 8713745868, Iran
    Iritaly Trading Company S.r.l., Via Volturno 58, 00185 Rome, Italy)

  • Luigi Schirone

    (School of Aerospace Engineering, Sapienza University of Rome, Via Salaria 851, 00138 Rome, Italy)

  • Mohammad Mahdi Abolhasani

    (Chemical Engineering Department, University of Kashan, Kashan 8731753153, Iran)

  • Narges Yaghoobi Nia

    (School of Aerospace Engineering, Sapienza University of Rome, Via Salaria 851, 00138 Rome, Italy
    Department of Electronics Engineering, University of Rome Tor Vergata, Via del Politecnico 1, 00133 Roma, Italy)

Abstract

Developing novel functional materials to advance the technological level of clean and renewable energy systems is the focus of much research. Due to their outstanding operational and compositional properties, perovskite-based structures have already been studied as an important class of solid-state components for electrochemical (EC), photoelectrochemical (PEC), and photovoltaic–electrochemical (PV-EC) CO 2 reduction, showing great potential in their catalytic activity and device stability and with a promising window for further technological developments. In this review, the different kinds of perovskites in the context of their structural features, which lead to their different applications, are first investigated. Then, we summarize the recent progress in the use of perovskites in EC, PEC, and PV-EC CO 2 -reduction devices. The research demonstrates that the mechanism and kinetics of intermediate formation have a significant effect on the creation of the final product. Investigations show that appropriate surface modifications, such as through the use of doping agents, alloy construction, and composites, can considerably improve the electrocatalytic activity and stability of perovskites. Finally, the perspectives on, and limitations of, the commercial and large-scale production of perovskites for CO 2 reduction are stated.

Suggested Citation

  • Mina Ahmadi-Kashani & Mahmoud Zendehdel & Luigi Schirone & Mohammad Mahdi Abolhasani & Narges Yaghoobi Nia, 2023. "Recent Progress in the Use of Perovskites for Electrochemical, Photoelectrochemical, and Photovoltaic–Electrochemical CO 2 Reduction," Energies, MDPI, vol. 16(22), pages 1-22, November.
    • Handle: RePEc:gam:jeners:v:16:y:2023:i:22:p:7632-:d:1282615
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    References listed on IDEAS

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    1. Hong Zhang & Kasra Darabi & Narges Yaghoobi Nia & Anurag Krishna & Paramvir Ahlawat & Boyu Guo & Masaud Hassan S. Almalki & Tzu-Sen Su & Dan Ren & Viacheslav Bolnykh & Luigi Angelo Castriotta & Mahmou, 2022. "A universal co-solvent dilution strategy enables facile and cost-effective fabrication of perovskite photovoltaics," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
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