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Experiments on surface light-induced drift for various systems

Author

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  • van der Meer, G.J.
  • Broers, B.
  • Hoogeveen, R.W.M.
  • Hermans, L.J.F.

Abstract

Surface light-induced drift of a low-pressure gas results from velocity-selective optical excitation combined with state-dependent molecule-surface interaction. This effect has been studied for CH3F and OCS, rovibrationally excited by a CO2 laser, interacting with various surfaces. For the R(4, 3) transition of 13CH3F, an increase in tangential momentum accommodation coefficient α upon excitation is found ranging from δα = 1.0 × 10-3 for stainless steel to δα = 14 × 10-3 for LiF(100) at 295 K. For this transition, the effect was also studied as a function of temperature for a quartz surface, resulting in a 40% decrease of δα as the temperature is raised from 300 to 700 K. Experiments for the P(5) transition of OCS yield δα = -0.53 × 10-3 on a quartz surface at 295 K.

Suggested Citation

  • van der Meer, G.J. & Broers, B. & Hoogeveen, R.W.M. & Hermans, L.J.F., 1992. "Experiments on surface light-induced drift for various systems," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 182(1), pages 47-58.
    • Handle: RePEc:eee:phsmap:v:182:y:1992:i:1:p:47-58
    DOI: 10.1016/0378-4371(92)90229-J
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